Conical Intersection Dynamics in NO <sub>2</sub> Probed by Homodyne High-Harmonic Spectroscopy

J. Wörner, H.; B. Bertrand, J.; Fabre, B.; Higuet, J.; Ruf, H.; Dubrouil, A.; Patchkovskii, S.; Spanner, M.; Mairesse, Y.; Blanchet, Valérie; Mével, E.; Constant, E.; B. Corkum, P.; M. Villeneuve, D.

doi:10.1126/science.1208664

Public

Conical Intersection Dynamics in NO 2 Probed by Homodyne High-Harmonic Spectroscopy

Published in Science • Oct 13, 2011

Authors:

H. J. Wörner

J. B. Bertrand

B. Fabre

Abstract

Conical intersections play a crucial role in the chemistry of most polyatomic molecules, ranging from the simplest bimolecular reactions to the photostability of DNA. The real-time study of the associated electronic dynamics poses a major challenge to the latest techniques of ultrafast measurement. ...

Subject

Conical intersection

Spectroscopy

Conical surface

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