Comprehensive study of carbon dioxide adsorption in the metal–organic frameworks M 2 (dobdc) (M = Mg, Mn, Fe, Co, Ni, Cu, Zn)

L. Queen, Wendy; R. Hudson, Matthew; D. Bloch, Eric; A. Mason, Jarad; I. Gonzalez, Miguel; S. Lee, Jason; Gygi, David; D. Howe, Joshua; Lee, Kyuho; A. Darwish, Tamim; R. James, Michael; K. Peterson, Vanessa; J. Teat, Simon; Smit, Berend; B. Neaton, Jeffrey; R. Long, Jeffrey; M. Brown, Craig

doi:10.1039/c4sc02064b

Public

Comprehensive study of carbon dioxide adsorption in the metal–organic frameworks M 2 (dobdc) (M = Mg, Mn, Fe, Co, Ni, Cu, Zn)

Published in Chemical Science • Aug 28, 2014

Authors:

Wendy L. Queen

Matthew R. Hudson

Eric D. Bloch

Abstract

Analysis of the CO2 adsorption properties of a well-known series of metal–organic frameworks M2(dobdc) (dobdc4− = 2,5-dioxido-1,4-benzenedicarboxylate; M = Mg, Mn, Fe, Co, Ni, Cu, and Zn) is carried out in tandem with in situ structural studies to identify the host–guest interactions that lead to si...

Subject

Adsorption

Intramolecular force

van der Waals force

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