Single Isolated Pd<sup>2+</sup> Cations Supported on N-Doped Carbon as Active Sites for Hydrogen Production from Formic Acid Decomposition

A. Bulushev, Dmitri; Zacharska, Monika; V. Shlyakhova, Elena; Chuvilin, Andrey; Guo, Yina; Beloshapkin, Sergey; V. Okotrub, A.; G. Bulusheva, Lyubov

doi:10.1021/acscatal.5b02381

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Single Isolated Pd2+ Cations Supported on N-Doped Carbon as Active Sites for Hydrogen Production from Formic Acid Decomposition

Published in ACS Catalysis • Dec 15, 2015

Authors:

Dmitri A. Bulushev

Monika Zacharska

Elena V. Shlyakhova

Abstract

Single-site heterogeneous catalysis with isolated Pd atoms was reported earlier, mainly for oxidation reactions and for Pd catalysts supported on oxide surfaces. In the present work, we show that single Pd atoms on nitrogen-functionalized mesoporous carbon, observed by aberration-corrected scanning ...

Subject

Catalysis

XANES

Formic acid

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