Semiconductive Copper(I)–Organic Frameworks for Efficient Light‐Driven Hydrogen Generation Without Additional Photosensitizers and Cocatalysts

Shi, Dongying; Zheng, Rui; Sun, Ming‐Jun; Cao, Xinrui; Sun, Chun‐Xiao; Cui, Chaojie; Liu, Chun‐Sen; Zhao, Junwei; Du, Miao

doi:10.1002/anie.201709869

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Semiconductive Copper(I)–Organic Frameworks for Efficient Light‐Driven Hydrogen Generation Without Additional Photosensitizers and Cocatalysts

Published in Angewandte Chemie International Edition • Sep 30, 2017

Authors:

Dongying Shi

Rui Zheng

Ming‐Jun Sun

Abstract

Abstract As the first example of a photocatalytic system for splitting water without additional cocatalysts and photosensitizers, the comparatively cost‐effective Cu2I2‐based MOF, Cu‐I‐bpy (bpy=4,4′‐bipyridine) exhibited highly efficient photocatalytic hydrogen production (7.09 mmol g−1 h−1). Densit...

Subject

Hydrogen production

Photocatalysis

Water splitting

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