Design of Single-Atom Co–N<sub>5</sub> Catalytic Site: A Robust Electrocatalyst for CO<sub>2</sub> Reduction with Nearly 100% CO Selectivity and Remarkable Stability

Pan, Yuan; Lin, Rui; Chen, Yinjuan; Liu, Shoujie; Zhu, Wei; Cao, Xing; Chen, Wenxing; Wu, Konglin; Cheong, Weng‐Chon; Wang, Yu; Zheng, Lirong; Luo, Jun; Lin, Yan; Liu, Yunqi; Liu, Chenguang; Li, Jun; Lu, Qi; Chen, Xin; Wang, Dingsheng; Peng, Qing; Chen, Chen; Li, Yadong

doi:10.1021/jacs.8b00814

Public

Design of Single-Atom Co–N5 Catalytic Site: A Robust Electrocatalyst for CO2 Reduction with Nearly 100% CO Selectivity and Remarkable Stability

Published in Journal of the American Chemical Society • Mar 8, 2018

Authors:

Yuan Pan

Rui Lin

Yinjuan Chen

Abstract

We develop an N-coordination strategy to design a robust CO2 reduction reaction (CO2RR) electrocatalyst with atomically dispersed Co–N5 site anchored on polymer-derived hollow N-doped porous carbon spheres. Our catalyst exhibits high selectivity for CO2RR with CO Faradaic efficiency (FECO) above 90%...

Subject

Chemistry

Electrocatalyst

Catalysis

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