Electroreduction of CO 2 on Single‐Site Copper‐Nitrogen‐Doped Carbon Material: Selective Formation of Ethanol and Reversible Restructuration of the Metal Sites

Karapinar, Dilan; Tran Huan, Ngoc; Ranjbar Sahraie, Nastaran; Li, Jingkun; Wakerley, David; Touati, Nadia; Zanna, Sandrine; Taverna, Dario; H. G. Tizei, Luiz; Zitolo, Andrea; Jaouen, Frédéric; Mougel, Victor; Fontecave, Marc

doi:10.1002/anie.201907994

Public

Electroreduction of CO 2 on Single‐Site Copper‐Nitrogen‐Doped Carbon Material: Selective Formation of Ethanol and Reversible Restructuration of the Metal Sites

Published in Angewandte Chemie International Edition • Aug 27, 2019

Authors:

Dilan Karapinar

Ngoc Tran Huan

Nastaran Ranjbar Sahraie

Abstract

Abstract It is generally believed that CO 2 electroreduction to multi‐carbon products such as ethanol or ethylene may be catalyzed with significant yield only on metallic copper surfaces, implying large ensembles of copper atoms. Here, we report on an inexpensive Cu‐N‐C material prepared via a simpl...

Subject

Copper

Faraday efficiency

Electrolysis

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