Activity Trends and Mechanisms in Peroxymonosulfate‐Assisted Catalytic Production of Singlet Oxygen over Atomic Metal‐N‐C Catalysts

Gao, Yun; Wu, Tongwei; Yang, Chengdong; Ma, Chao; Zhao, Zhenyang; Wu, Zihe; Cao, Sujiao; Geng, Wei; Wang, Yi; Yao, Yongyi; Zhang, Yanning; Cheng, Chong

doi:10.1002/anie.202109530

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Activity Trends and Mechanisms in Peroxymonosulfate‐Assisted Catalytic Production of Singlet Oxygen over Atomic Metal‐N‐C Catalysts

Published in Angewandte Chemie International Edition • Aug 13, 2021

Authors:

Yun Gao

Tongwei Wu

Chengdong Yang

Abstract

Abstract We synthesized a series of carbon‐supported atomic metal‐N‐C catalysts (M‐SACs: M=Mn, Fe, Co, Ni, Cu) with similar structural and physicochemical properties to uncover their catalytic activity trends and mechanisms. The peroxymonosulfate (PMS) catalytic activity trends are Fe‐SAC>Co‐SAC>Mn‐...

Subject

Catalysis

Chemistry

Singlet oxygen

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